透视图(图形)
电化学
催化作用
可再生能源
电化学能量转换
生化工程
能量转换
计算机科学
材料科学
纳米技术
化学
工程类
电气工程
电极
物理
有机化学
人工智能
物理化学
热力学
作者
Florian Speck,Jae Hyung Kim,Geunsu Bae,Sang Hoon Joo,Karl J. J. Mayrhofer,Chang Hyuck Choi,Serhiy Cherevko
出处
期刊:JACS Au
[American Chemical Society]
日期:2021-06-21
卷期号:1 (8): 1086-1100
被引量:83
标识
DOI:10.1021/jacsau.1c00121
摘要
Single-atom catalysts (SACs) hold great promise for maximized metal utilization, exceptional tunability of the catalytic site, and selectivity. Moreover, they can substantially contribute to lower the cost and abundancy challenges associated with raw materials. Significant breakthroughs have been achieved over the past decade, for instance, in terms of synthesis methods for SACs, their catalytic activity, and the mechanistic understanding of their functionality. Still, great challenges lie ahead in order to render them viable for application in important fields such as electrochemical energy conversion of renewable electrical energy. We have identified three particular development fields for advanced SACs that we consider crucial, namely, the scale-up of the synthesis, the understanding of their performance in real devices such as fuel cells and electrolyzers, and the understanding and mitigation of their degradation. In this Perspective, we review recent activities of the community and provide our outlook with respect to the aspects required to bring SACs toward application.
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