石墨烯
石墨氮化碳
材料科学
光降解
化学工程
氧化物
水溶液
光催化
饮用水净化
碳纤维
吸附
复合材料
纳米技术
化学
有机化学
冶金
复合数
催化作用
工程类
作者
Mahdi Karimi‐Nazarabad,Elaheh K. Goharshadi,Roya Mehrkhah,Maryam Davardoostmanesh
标识
DOI:10.1016/j.seppur.2021.119788
摘要
Herein, a multifunction system was designed for water purification. Reduced graphene oxide (RGO) and graphitic carbon nitride (g-C3N4) nanosheets were deposited on poplar wood to prepare the double-layer multifunctional nanoplatforms for use in a solar steam generation (SSG) of seawater, photodegradation of an organic pollutant (RB5 azo dye), and sorption of Pb (II) from aqueous solutions. The solar steam flux of 4.78 kg m−2h−1 was achieved by RGO/g-C3N4/wood under 3 kW m−2, respectively. High performance of RGO/g-C3N4/wood device is due to the broadband harvesting of solar energy of RGO/g-C3N4 as a photothermal material and channeled structure, low thermal conductivity (TC), and hydrophilic nature of wood as a substrate. The durability test showed a stable performance of RGO/g-C3N4/wood photoabsorber for 30 cycles. The total cost of solar water evaporation of RGO4/g-C3N4/wood was calculated to be 0.08 USD/(cm3 h−1) which is significantly more cost-effective than other previous reports. RGO/g-C3N4/wood as an efficient photocatalyst degraded completely RB5. g-C3N4 plays the main role in the photodegradation of dye and RGO improves its photocatalytic performance by slowing the electron/hole recombination. Also, RGO/g-C3N4/wood as a sorbent adsorbed completely Pb (II) from aqueous solutions.
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