微等离子体
甲醇
能量转换
能量转换效率
材料科学
化学工程
等离子体
工艺工程
环境科学
纳米技术
化学
光电子学
有机化学
工程类
物理
热力学
量子力学
作者
Jin Ru,Qi Wu,Hong‐Ping He,Changhua Wang,Yuanyuan Li,Dexin Jin,Shuang Liang,He Ma,Dashuai Li,Rui Wang,Yingying Li,Xintong Zhang
标识
DOI:10.1002/smtd.202401704
摘要
Abstract The clean conversion of CO 2 is a strategic issue for addressing global climate change and advancing energy transformation. While the current clean CO 2 conversion is limited to the H 2 pyrolysis process, using H 2 O as a proton source is more promising and sustainable. A microplasma discharge method is developed, driven by electricity, and utilized for CO 2 conversion with H 2 O. The microplasma integrates the advantages of high energy density in discharge plasma and microchannel reaction spaces, achieving a rapid resource conversion process of CO 2 and water and a high selectivity for methanol production. By further combining In 2 O 3 with microplasma and optimizing the structure of In 2 O 3 , is improved the selectivity of methanol production to 86.66%. The methanol production rate reached 72.64 mmol g −1 h − ¹, which is higher than other clean energy‐driven conversion technologies. This work provides a green route for uphill reactions in clean CO 2 conversion, offering a new approach for CO 2 emission reduction and resource utilization.
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