制氢
耐久性
电解
聚合物电解质膜电解
氢
工艺工程
电解水
环境科学
纳米技术
化学工程
化学
材料科学
电极
工程类
有机化学
物理化学
电解质
复合材料
作者
Begüm Yarar Kaplan,Ahmet Can Kırlıoğlu,Mohammad Alinezhadfar,Mohammed Ahmed Zabara,Naeimeh Rajabalizadeh Mojarrad,Bilal Iskandarani,Alp Yürüm,Cengiz S. Ozkan,Mihrimah Ozkan,Selmiye Alkan Gürsel
出处
期刊:Chem catalysis
[Elsevier]
日期:2023-05-01
卷期号:3 (5): 100601-100601
标识
DOI:10.1016/j.checat.2023.100601
摘要
For deep decarbonization, pressure is on to develop better green hydrogen energy sources with higher efficiency, extended durability, and lower cost. Electrolysis is very promising for green hydrogen production, yet several challenges need to be overcome. Operando techniques can offer in situ monitoring and real-time observation of water electrolysis, including reaction mechanisms, structural changes, ionic conductivity, transport properties, and degradation mechanisms. We first discuss the current progress in operando analysis of electrolysis for hydrogen production and provide an overview of recent advances in radiography and tomography techniques: infrared, Raman, X-ray absorption, photoelectron, and electrochemical impedance spectroscopy methods. Next, operational principles; temporal, spatial, and spectral ranges; and limitations in operando monitoring and analyses are presented. Furthermore, reactions and mechanisms that occur in these systems, and resultant system durability, are reviewed. Finally, we recommend future directions in operando characterization for enhancing live monitoring of reactions, transport phenomena, and degradation mechanisms in hydrogen production.
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