纳滤
膜
Zeta电位
傅里叶变换红外光谱
化学
X射线光电子能谱
核化学
扫描电子显微镜
化学工程
材料科学
纳米颗粒
生物化学
工程类
复合材料
作者
Xuehai Yan,Shirong Cheng,Cong Ma,Junyu Li,Guodong Wang,Chengyu Yang
标识
DOI:10.1016/j.jhazmat.2021.126939
摘要
Sodium tetraborate pentahydrate (STB) was intercalated into graphene oxide (GO) nanosheets to form a nanocomposite ([email protected]). Subsequently, it was self-assembled on a substrate membrane to prepare [email protected] nanofiltration membrane. The properties of the [email protected] powder samples and the nanofiltration membrane were studied using scanning electron microscopy (SEM), Fourier transform infrared spectroscopy (FTIR), X-ray photoelectron spectroscopy (XPS), X-ray diffraction (XRD), contact angle (CA), and zeta potential. When the STB concentration was 1.0 g/L in the cross-linking reaction, the membrane was described as the STB2@GO membrane and exhibited a large interlayer space (d-spacing = 1.347 nm), high hydrophilicity (CA = 22.2°), and high negative potential (zeta = −18.0 mV). Meanwhile, the pure water flux of the membrane was significantly increased by 56.60% than that of the GO membrane. In addition, the STB2@GO membrane exhibited a favorable capability for dye rejection,98.52% for Evans blue (EB), 99.26% for Victoria blue B (VB), 91.94% for Alizarin yellow (AY), and 93.21% for Neutral red (NR). Furthermore, the STB2@GO membrane performed better in dye separation under various types and concentrations of dye, pH values, and ions in solution. Thus, this study provides a promising method for preparing laminated GO nanofiltration membranes for dye wastewater treatment.
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