接触角
水溶液
润湿
超疏水涂料
纳米颗粒
表面改性
作者
Yong Xu,Gang Wang,Lijing Zhu,Luli Shen,Zhepeng Zhang,Tianhui Ren,Zhixiang Zeng,Tao Chen,Qunji Xue
标识
DOI:10.1016/j.jhazmat.2020.124374
摘要
Abstract Supra-wetting materials, especially superhydrophobic absorption materials, as an emerging advanced oil-water separation material have attracted extensive concern in the treatment of oil spillage and industrial oily wastewater. However, it is still a challenge to fabricate robust and multifunctional superhydrophobic materials for the multitasking oil-water separation and fast clean-up of the viscous crude oil by an environment-friendly and scalable method. Herein, a solid-solid phase ball-milling strategy without chemical reagent-free modification was proposed to construct heterogeneous superhydrophobic composites by using waste soot as the solid-phase superhydrophobic modifier. A series of covalent bond restricted soot-graphene (S-GN) or soot-Fe3O4 (S-Fe3O4) composite materials with a peculiar micro-nano structure are prepared. Through glue+superhydrophobic method, the prepared soot-based composite particles are facilely loaded on the porous skeleton of the sponge to obtain multifunctional superhydrophobic adsorbents. The reported superhydrophobic adsorbents exhibited robust chemical and mechanical stability, convenient magnetic collection, the high oil absorption capacity of 60–142 g g−1, durable recyclability (>250 cycles), efficient separation efficiency (>99.5%) and outstanding self-heated performance, which enable them to be competent for oil-water separation in multitasking and complex environment (floating oils, continuous oil collection, oil-in-water emulsion, and viscous oil-spills).
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