微生物燃料电池
阳极
阴极
材料科学
功率密度
电极
层流
电解质
纳米技术
碳纳米管
电流密度
光电子学
化学工程
化学
功率(物理)
工程类
量子力学
物理
物理化学
航空航天工程
作者
Cheon Ho Lee,Hongyoung Ha,Yoomin Ahn,Hong Liu
标识
DOI:10.1016/j.jpowsour.2023.233456
摘要
This paper presents a novel design and operation of microbial fuel cells (ΜFCs), which contain monolayer paper-based substrate/electrodes and microchannels with co-laminar flow. The electrodes with multi-wall carbon nanotubes are fabricated by the screen-printing method and the microchannels are patterned using photo-lithography. A double-inlet and diverging channel design is incorporated in the fuel cell configuration and demonstrated significantly improved performance. The fluid flows of electrolytes through the porous paper media are simulated using steady-state and transient computational fluid dynamics The best performance is achieved under the following conditions: an electroactive microbial (S. oneidensis) concentration of OD6001.5, 50 mM electron donor (lactate), and direct immobilized of the inoculum on the anode surface. The developed MFCs achieves a peak power density of 19.4 ± 0.23 μW cm−2 and maximum current density of 190.4 ± 1.39 μA cm−2, surpassing the performance of all previously reported paper-based single MFCs that utilize paper-based electrodes. In addition, hybrid-type MFCs that containing enzymatic air-breathing cathodes are investigated to enhance their performance. The novel paper based self-pumping MFC has the potential to make lab-on-a-chip type portable medical diagnosis devices with integrated power sources practical and feasible.
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