Laminated magnetic graphene with enhanced electromagnetic wave absorption properties

材料科学 石墨烯 反射损耗 电磁辐射 微波食品加热 电介质 介电损耗 吸收(声学) 复合材料 复合数 光电子学 光学 纳米技术 量子力学 物理
作者
Xin Sun,Jianping He,Guoxian Li,Jing Tang,Tao Wang,Yunxia Guo,Hairong Xue
出处
期刊:Journal of Materials Chemistry C [Royal Society of Chemistry]
卷期号:1 (4): 765-777 被引量:737
标识
DOI:10.1039/c2tc00159d
摘要

Graphene is highly desirable as an electromagnetic wave absorber because of its high dielectric loss and low density. Nevertheless, pure graphene is found to be non-magnetic and contributes to microwave energy absorption mostly because of its dielectric loss, and the electromagnetic parameters of pure graphene, which are out of balance, result in a bad impedance matching characteristic. In this paper, we report a facile solvothermal route to synthesize laminated magnetic graphene. The results show that there have been significant changes in the electromagnetic properties of magnetic graphene when compared with pure graphene. Especially the dielectric Cole–Cole semicircle suggests that there are Debye relaxation processes in the laminated magnetic graphene, which prove beneficial to enhance the dielectric loss. We also proposed an electromagnetic complementary theory to explain how laminated magnetic graphene, with the combined advantages of graphene and magnetic particles, helps to improve the standard of impedance matching for electromagnetic wave absorbing materials. Besides, microwave absorption properties indicate that the reflection loss of the as-prepared composite is below −10 dB (90% absorption) at 10.4–13.2 GHz with a coating layer thickness of 2.0 mm. This further confirms that the nanoscale surface modification of magnetic particles on graphene makes graphene-based composites have a certain research value in electromagnetic wave absorption.
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