分析物
信号(编程语言)
化学
检出限
多菌灵
压力传感器
软件可移植性
压阻效应
色谱法
光电子学
计算机科学
材料科学
工程类
植物
杀菌剂
机械工程
生物
程序设计语言
作者
Jinxia Xue,Honglin Yang,Jizhou Li,Hui Ouyang,Zhifeng Fu
标识
DOI:10.1021/acs.analchem.2c04322
摘要
Pressure has been a facile signal readout mode for developing point-of-care testing devices due to the attractive features of portability, accessibility, rapidity, and affordability. Herein, a pressure signal readout device was designed by integrating two homemade needle-type piezoresistive transducers, a controller for a thin-film piezoresistive sensor and a smartphone. Meanwhile, a bidirectional immunochromatographic test strip was designed as an immunoreaction platform for dual-analyte detection. Using PdCuPt nanoparticles with catalase-mimic activity as signal tags, the pressure signals triggered by catalyzed aerogenous reaction were monitored by the pressure signal readout device and read on a smartphone with the Bluetooth module. In this proof-of-principle work, imidacloprid and carbendazim were detected as model analytes. The dynamic ranges for quantitating imidacloprid and carbendazim are 20 pg mL-1 to 50 ng mL-1 and 50 pg mL-1 to 50 ng mL-1, respectively. The whole immunoassay process was completed within 16 min. The recovery values for imidacloprid and carbendazim spiked into herbal medicines are 82.0-110.0 and 84.0-116.0%, respectively, verifying its reliability for real sample detection. As the smartphone APP and controller for a thin-film piezoresistive sensor contain 12 signal channels, the system can be easily extended to meet the demand for high-throughput screening.
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