Hydrogen-mediated control of magnetic anisotropy and magnetic domain structure in Co/Pd multilayer

This study demonstrates the reversible transition from perpendicular to in-plane magnetic anisotropy in Co/Pd multilayers induced by hydrogenation, using a magneto-optic Kerr microscope. By controlling hydrogen pressure and exposure time, the transition is separated into coercivity and squareness ratio changes, reflecting reduced perpendicular anisotropy and spin reorientation. The Dzyaloshinskii–Moriya interaction is observed through asymmetric magnetic domain expansion, with hydrogenation causing domains to fragment. These results suggest hydrogenation as a method for precise control of magnetic anisotropy and domain structures.