光催化
分解水
纳米复合材料
催化作用
制氢
罗丹明B
材料科学
硒化物
硒化锌
化学工程
纳米技术
无机化学
化学
冶金
硒
生物化学
光电子学
工程类
作者
Harshavardhan Mohan,Ga Hyeon Ha,Hyeon Seung Oh,Gitae Kim,Taeho Shin
出处
期刊:Chemosphere
[Elsevier]
日期:2022-11-01
卷期号:307: 135937-135937
被引量:10
标识
DOI:10.1016/j.chemosphere.2022.135937
摘要
Hydrogen has been considered as a promising clean energy source owing to its renewability and zero carbon emission. Accordingly, photocatalytic water splitting has drawn much attention as a key green technology of producing hydrogen. However, it has remained as a great challenge due to the low production rate and expensive constituents of photocatalytic systems. Herein, we synthesised nanostructures consisting of transition metal selenide and g-C3N4 for photocatalytic water splitting reaction. They include ZnSe, FeSe2, Zn/FeSe2 and ZnFeSe2 nanoflowers and a nanocomposite made of Zn/FeSe2 and g-C3N4. Hydrogen evolution rates in the presence of ZnSe, FeSe2, Zn/FeSe2 and ZnFeSe2 photocatalysts were measured as 60.03, 128.02, 155.11 and 83.59 μmolg-1 min-1, respectively. On the other hand, with the nanocomposite consisting of Zn/FeSe2 and g-C3N4, the hydrogen and oxygen evolution rates were significantly enhanced up to 202.94 μmol g-1min-1 and 90.92 μmol g-1min-1, respectively. The nanocomposite was also examined as a photocatalyst for degradation of rhodamine B showing that it photodegrades the compound two times faster compared to pristine Zn/FeSe2 nanoflowers without g-C3N4. Our study suggests the nanocomposite of Zn/FeSe2 and g-C3N4 as a promising photocatalyst for energy and environmental applications.
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