High-performance quasi-2D perovskite solar cells enabled by using π-conjugated spacer

The excellent photoelectric properties and low fabrication cost of perovskite solar cells have attracted extensive research attention. Despite this, long-term stability issues associated with perovskite solar cells continue to pose a significant barrier to commercialization. A new generation of two-dimensional (2D) and quasi-2D perovskites and newly introduced members of the 2D material family, have attracted growing attention due to their excellent stability and physical properties in contrast to their three-dimensional (3D) counterparts. Herein, we have presented the feasibility of using 4,4[Formula: see text]-dipyridyl as an additive material for quasi-2D perovskite solar cells. As a result of the addition of 4,4[Formula: see text]-dipyridyl, the solar cell device achieves a power conversion efficiency of 17.92% and a fill factor of 76.5%. Additionally, this strategy can be expanded to quasi-2D perovskite solar cells with an open-circuit voltage of 1.05[Formula: see text]V.