Ultrasensitive polarization-dependent terahertz modulation in hybrid perovskites plasmon-induced transparency devices

Active control of metamaterial properties with high tunability of both resonant intensity and frequency is essential for advanced terahertz (THz) applications, ranging from spectroscopy and sensing to communications. Among varied metamaterials, plasmon-induced transparency (PIT) has enabled active control with giant sensitivity by embedding semiconducting materials. However, there is still a stringent challenge to achieve dynamic responses in both intensity and frequency modulation. Here, an anisotropic THz active metamaterial device with an ultrasensitive modulation feature is proposed and experimentally studied. A radiative-radiative-coupled PIT system is established, with a frequency shift of 0.26 THz in its sharp transparent windows by polarization rotation. Enabled by high charge-carrier mobility and longer diffusion lengths, we utilize a straightforwardly spin-coated MAPbI3 film acting as a photoactive medium to endow the device with high sensitivity and ultrafast speed. When the device is pumped by an ultralow laser fluence, the PIT transmission windows at 0.86 and 1.12 THz demonstrate a significant reduction for two polarizations, respectively, with a full recovery time of 561 ps. In addition, we numerically prove the validity that the investigated resonator structure is sensitive to the optically induced conductivity. The hybrid system not only achieves resonant intensity and frequency modulations simultaneously, but also preserves the all-optical-induced switching merits with high sensitivity and speed, which enriches multifunctional subwavelength metamaterial devices at THz frequencies.