Atomically Thin Synaptic Devices for Optoelectronic Neuromorphic Vision

Abstract Imaging sensors with inbuilt processing capability are expected to form the backbone of low‐latency and highly energy efficient artificial vision systems. A range of emerging atomically thin materials provide opportunities to exploit their electrical and optical properties for human vision and brain inspired functions. This work reports atomically thin nanosheets of β‐In 2 S 3 which exhibit inherent persistent photoconductivity (PPC) under ultraviolet and visible wavelengths. This PPC effect enables β‐In 2 S 3 ‐based optoelectronic devices to optically mimic the dynamics of biological synapses. Based on the material characterizations, the PPC effect is attributed to the intrinsic defects in the synthesized β‐In 2 S 3 nanosheet. Furthermore, the feasibility of adopting these atomically thin synaptic devices for optoelectronic neuromorphic hardware is demonstrated by implementing a convolutional neural network for image classification. As such, the demonstrated atomically thin nanosheets and optoelectronic synaptic devices provide a platform for scaling up complex vision‐sensory neural networks, which can find many promising applications for multispectral imaging and neuromorphic computation.