Li-Ion Doped Artificial Synaptic Memristor for Highly Linear Neuromorphic Computing

Linear weights modulation in neuromorphic memristor plays an important role in high-accuracy image recognition task. Herein, a Li+ doped organic artificial memristor for neuromorphic computing was proposed for linear weights update, which shows active ions diffusive dynamics as Ca2+ diffusion in biological synapse. The memristor exhibits gradual resistive switching, multi-state storage and typical synaptic behaviors. In addition, the synaptic learning capability of letter "T" was demonstrated in a memristors array. By designing consecutive pulse waveforms with enhanced amplitude, the linearity of memristor for weight update in long-term potentiation and depression (LTP/LTD) could be improved from 6.8 to 0.4. Based on the great nonlinearity factor in LTP ( $\alpha _{\text {p}}={1.5}$ ) and LTD ( $\alpha _{\text {d}}={0.4}$ ), face recognition was achieved with high accuracy of 96% by artificial neural network consisting of ion doped memristors. The ion doped organic memristor with highly linear weights update provides guidelines for the development of bio-inspired ion diffusive neuromorphic computing system.