Magnetism and charge density wave order in kagome FeGe

磁性 物理 凝聚态物理 电荷密度波 角分辨光电子能谱 电子结构 费米能级 拓扑绝缘体 电子能带结构 电子 格子(音乐) 超导电性 量子力学 声学
作者
Xiaokun Teng,Ji Seop Oh,Hengxin Tan,Lebing Chen,Jianwei Huang,Bin Gao,Jia‐Xin Yin,Jiun‐Haw Chu,Makoto Hashimoto,Dong-Hui Lu,Chris Jozwiak,Aaron Bostwick,Eli Rotenberg,G. E. Granroth,Binghai Yan,R. J. Birgeneau,Pengcheng Dai,Ming Yi
出处
期刊:Nature Physics [Nature Portfolio]
卷期号:19 (6): 814-822 被引量:102
标识
DOI:10.1038/s41567-023-01985-w
摘要

Electron correlations often lead to emergent orders in quantum materials. Kagome lattice materials are emerging as an exciting platform for realizing quantum topology in the presence of electron correlations. This proposal stems from the key signatures of electronic structures associated with its lattice geometry: flat band induced by destructive interference of the electronic wavefunctions, topological Dirac crossing, and a pair of van Hove singularities (vHSs). A plethora of correlated electronic phases have been discovered amongst kagome lattice materials, including magnetism, charge density wave (CDW), nematicity, and superconductivity. These materials can be largely organized into two types: those that host magnetism and those that host CDW order. Recently, a CDW order has been discovered in the magnetic kagome FeGe, providing a new platform for understanding the interplay between CDW and magnetism. Here, utilizing angle-resolved photoemission spectroscopy, we observe all three types of electronic signatures of the kagome lattice: flat bands, Dirac crossings, and vHSs. From both the observation of a temperature-dependent shift of the vHSs towards the Fermi level as well as guidance via first-principle calculations, we identify the presence of the vHSs near the Fermi level (EF) to be driven by the development of underlying magnetic exchange splitting. Furthermore, we show spectral evidence for the CDW order as gaps that open on the near-EF vHS bands, as well as evidence of electron-phonon coupling from a kink on the vHS band together with phonon hardening observed by inelastic neutron scattering. Our observation points to the magnetic interaction-driven band modification resulting in the formation of the CDW order, indicating an intertwined connection between the emergent magnetism and vHS charge order in this moderately-correlated kagome metal.
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