Realization of 3D epoxy resin/Ti3C2T x MXene aerogel composites for low-voltage electrothermal heating

Abstract Suitable electrothermal materials with high heating rates at low electric power are highly desirable for de-icing and thermal management applications. Herein, 3D epoxy resin/Ti 3 C 2 T x MXene composites are synthesised and shown to be promising candidates for electrothermal heaters where the MXene serves as a nanoheater and the epoxy resin spreads the heat. A unidirectional freeze-casting technique was used to prepare an anisotropic Ti 3 C 2 T x aerogel into which epoxy resin was then vacuum infiltrated and cured. The resulting composite showed an excellent Joule heating performance over repeated heating–cooling cycles. A steady-state temperature of 123 °C was obtained by applying a low voltage of 2 V with 5.1 A current, giving a total power output of 6.1 W cm −2 . Such epoxy/MXene aerogel composites, prepared by a simple and cost-effective manner, offer a potential alternative to the traditional metal-based and nanocarbon-based electrothermal materials.