超级电容器
材料科学
电容
石墨烯
纳米技术
制作
微流控
纺纱
纤维
电极
储能
多孔性
光电子学
复合材料
功率(物理)
化学
物理
医学
病理
物理化学
量子力学
替代医学
作者
Yunming Jia,Xiaying Jiang,Arsalan Ahmed,Lan Zhou,Qinguo Fan,Jianzhong Shao
出处
期刊:Journal of The Electrochemical Society
[The Electrochemical Society]
日期:2021-07-01
卷期号:168 (7): 070514-070514
被引量:4
标识
DOI:10.1149/1945-7111/ac0f85
摘要
Fiber-shaped supercapacitors are desirable candidates for flexible and wearable energy storage devices; however, the ultralow capacitance and intricate fabrication process of electrode materials significantly limits their performances. We exploited a steerable method to generate core–shell α-MnO2/graphene fibers (MnGFs), where the sheath of α-MnO2 with porous network structures were grown in situ intertwined on the core of graphene fiber in a microfluidic-spinning strategy. The as-obtained MnGFs exhibited outstanding mechanical flexibility and could be curled over a teflon rod for continuous production. Furthermore, the fiber-shaped supercapacitors (MGSCs) manufactured with MnGFs were successfullu assembled and exhibited good voluminal specific capacitance (136.7 F cm−3), prominent cyclic stability (91.6% retention over 10000 cycles), and high energy density (3.9 mWh cm−3). This advantageous performance was achieved by MnGFs with porous network structures, leading to the rich ion pseudo-capacitance and numerous electron transport channels. The as-prepared MGSCs could be easily adopted to power 5 light-emitting diodes after completel charging. We believe that our microfluidic spinning strategy can provide a new-style structural design method for efficient electrode materials and promote the progress of wearable electronic products.
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