Plasmonic random laser from dye-doped cholesteric liquid crystals incorporating silver nanoprisms

Plasmonic random lasers have been demonstrated in combining dye-doped cholesteric liquid crystals (DD-CLCs) and silver nanoparticles (AgNPs). The DD-CLC laser reveals the lowest threshold and highest slope efficiency through the localized surface plasmon resonance of AgNPs with the best coupling of the emission spectrum of lasing dye and resonance of electron oscillation on the metal surface. Thermal control of the DD-CLC lasers has been achieved to simultaneously shift the long- and short-edge lasing peaks. By the α -stable analysis, the DD-CLC random laser (RL) reveals heavy tail distribution with relatively low α ∼ 1.06 to show the Lévy behavior. Owing to its low spatial coherence, the DD-CLC RL has been demonstrated to produce a speckle-reduced image with a lower contrast of about 0.04.