固体表面
水溶液
微流控
化学
地表水
流量(数学)
化学物理
纳米技术
水流
化学工程
材料科学
物理化学
物理
机械
环境科学
环境工程
工程类
作者
Dan Lis,Ellen H. G. Backus,Johannes Hunger,Sapun H. Parekh,Mischa Bonn
出处
期刊:Science
[American Association for the Advancement of Science (AAAS)]
日期:2014-06-06
卷期号:344 (6188): 1138-1142
被引量:184
标识
DOI:10.1126/science.1253793
摘要
Monitoring water interfaces in motion Water behaves differently at interfaces—where it meets the air, or a solid surface—than it does in the middle of the liquid. Past laboratory studies of this phenomenon have mainly focused on still samples, despite the fact that in natural settings such as rivers and rain, the water moves along the surfaces. Lis et al. used a microfluidics apparatus and a spectroscopy technique called sum frequency generation to study the effects of flow on aqueous chemistry at silica and fluorite surfaces (see the Perspective by Waychunas). The flow of fresh water along the surfaces disrupts the equilibrium of dissolved ions, substantially changing the surface charge and the molecular orientation of the water at the interface. Science , this issue p. 1138 ; see also p. 1094
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