吸附
制作
材料科学
检出限
纳米技术
电极
信号(编程语言)
氨
选择性
水准点(测量)
响应时间
光电子学
计算机科学
化学
色谱法
有机化学
医学
替代医学
计算机图形学(图像)
物理化学
病理
大地测量学
程序设计语言
地理
催化作用
作者
Sa Wang,Yu Fu,Ting Wang,Wansheng Liu,Jian Wang,Peng Zhao,Heping Ma,Yao Chen,Peng Cheng,Zhenjie Zhang
标识
DOI:10.1038/s41467-023-42959-z
摘要
Abstract The development of fast-response sensors for detecting NH 3 at room temperature remains a formidable challenge. Here, to address this challenge, two highly robust Hoffmann-type metal-organic frameworks are rationally applied as the NH 3 sensing materials which possess ultra-high static adsorption capacity for NH 3 , only lower than the current benchmark material. The adsorption mechanism is in-depth unveiled by dynamic adsorption and simulation studies. The assembled interdigital electrode device exhibits low detection limit (25 ppb) and short response time (5 s) at room temperature, which set a record among all electrical signal sensors. Moreover, the sensor exhibits excellent selectivity towards NH 3 in the presence of 13 other potential interfering gases. Prominently, the sensor can stably output signals for more than two months at room temperature and can be recovered by simply purging nitrogen at room temperature without heating. This study opens up a way for reasonably designing gas sensing materials for toxic gases.
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