A Solution‐Processed Resonance Host for Highly Efficient Electrophosphorescent Devices with Extremely Low Efficiency Roll‐off

Solution-processible N–P=O resonance-host molecules are applied successfully in spin-coated phosphorescent light-emitting diodes (PHOLEDs) to selectively and self-adaptively tune the electrical properties for balanced charge transportation. The resonance-molecule-hosted PHOLEDs exhibit a high maximum quantum efficiency of 16.5% and a low efficiency roll-off down to 0.7%, highlighting the significant progress of these solution-processed PHOLEDs with high efficiency and flat efficiency roll-off achieved simultaneously. As a service to our authors and readers, this journal provides supporting information supplied by the authors. Such materials are peer reviewed and may be re-organized for online delivery, but are not copy-edited or typeset. Technical support issues arising from supporting information (other than missing files) should be addressed to the authors. Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article.