催化作用
析氧
过电位
化学工程
电催化剂
碳纤维
材料科学
碳化
纳米棒
无机化学
化学
纳米技术
电化学
有机化学
复合材料
物理化学
电极
工程类
复合数
扫描电子显微镜
作者
Yumin Ye,Xin Zhao,Changwei Li,Zongshun Zhang,Huixin Zhang,Junliu Zhang,Shenghui Jiao,Honglei Chen
标识
DOI:10.1016/j.mcat.2023.113579
摘要
The oxygen evolution reaction (OER) process in water electrolysis requires high energy consumption. Reducing the interface limitations between metal and carbon precursors can significantly enhance the catalytic performance during the OER process. Because biomass exists in solid form, in this work, a carbon-coated Na/Fe@C nanorod OER electrocatalyst using soybean straw was prepared by coupling polyethylene glycol green liquefaction, in-situ doping, and carbonization route. The carbon coating increased the surface area and active site of the catalyst and prevented catalyst oxidation, thus extending the lifespan of the catalyst. The Na/Fe@C catalysts exhibited excellent OER catalytic activity. The overpotential at a current density of 10 mA cm−2 and 100 mA cm−2 were 275 and 320 mV, respectively. Therefore, this study provides a promising strategy for preparing stable electrocatalysts and reducing OER energy consumption.
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