Inkjet-Printed Full-Color Matrix Quasi-Two-Dimensional Perovskite Light-Emitting Diodes

Full-color matrix devices based on perovskite light-emitting diodes (PeLEDs) formed via inkjet printing are increasingly attractive due to their tunable emission, high color purity, and low cost. A key challenge for realizing PeLED matrix devices is achieving high-quality perovskite films with a favorable emission structure via inkjet printing techniques. In this work, a narrow phase distribution, high-quality quasi-two-dimensional (quasi-2D) perovskite film without a "coffee ring" was obtained via the introduction of a phenylbutylammonium cation into the perovskite and the use of a vacuum-assisted quick-drying process. Relatively efficient emissions of red, green, and blue (RGB) uniform quasi-2D perovskite films with high photoluminescence quantum yields were cast by the inkjet printing technique. The RGB monochrome perovskite matrix devices with 120 pixel-per-inch resolution exhibited electroluminescence, with maximum external quantum efficiencies of 3.5, 3.4, and 1.0% (for red, green, and blue light emissions, respectively). Furthermore, a full-color perovskite matrix device with a color gamut of 102% (NTSC 1931) was realized. To the best of our knowledge, this is the first report of a full-color perovskite matrix device formed by inkjet printing.