Giant Electrical Modulation of Terahertz Emission in Pb(Mg1/3Nb2/3)0.7

Spintronic terahertz (THz) emitters based on ferromagnetic (FM)-nonmagnetic (NM) heterostructures are the focus of many experimental endeavors for THz sources. However, existing spintronic THz sources control emission by changing the external magnetic field, which is inconvenient for compact integration. Therefore, various modulated mechanisms are in high demand. Here, we present an electric-field-controlled spintronic THz emitter based on the ferroelectric (FE)-FM/NM structure that can emit THz radiation with voltage-modulated amplitude and polarization angle. The modulation depth of the THz amplitude is up to 69%, and the maximum rotation of the THz polarization angle is 28\ifmmode^\circ\else\textdegree\fi{}. In addition, after removing the electric field, two different THz-emission states can remain unchanged, demonstrating nonvolatile behavior. Modulation is attributed to magnetoelectric coupling between the FM and FE layers, which modifies magnetization of the FM layer by the electric-field-induced strain in the FE layer, and thus, modulates THz emission. Furthermore, the possibility of a programmable array-type THz source with varied bias voltage is theoretically demonstrated, allowing a spatially modulated THz light to be generated directly without the use of additional spatial light modulators. We believe that this electric-field-controlled THz emitter has the potential to be used in next-generation on-chip THz sources, THz memory devices, and THz ghost imaging.