Efficient Generation of a Near-visible Frequency Comb via Cherenkov-like Radiation from a Kerr Microcomb

Optical frequency combs enable state-of-the-art applications including frequency metrology, optical clocks, astronomical measurements, and sensing. Recent demonstrations of microresonator-based Kerr frequency combs or microcombs pave the way to scalable and stable comb sources on a photonic chip. Generating microcombs in the visible wavelength range, however, has been limited by large material dispersion and optical loss. Here we demonstrate a scheme for efficiently generating visible microcomb in a high Q aluminum nitride microring resonator. Enhanced Pockels effect strongly couples infrared and visible modes into hybrid mode pairs, which participate in the Kerr microcomb generation process and lead to strong Cherenkov radiation in the visible band of an octave apart. A surprisingly high conversion efficiency of 22% is achieved from the pump laser to the visible comb. We further demonstrate a robust frequency tuning of the visible comb by more than one free spectral range and apply it to the absorption spectroscopy of a water-based dye molecule solution. Our work marks the first step towards high-efficiency visible microcomb generation and its utilization, and it also provides insights on the significance of Pockels effect and its strong coupling with Kerr nonlinearity in a single microcavity device.