环境友好型
磷酸铁锂
再生(生物学)
环境科学
废物管理
锂(药物)
原材料
环境污染
材料科学
污染物
电池(电)
功率(物理)
工程类
化学
环境保护
有机化学
生态学
量子力学
医学
内分泌学
物理
细胞生物学
生物
作者
Xiaohui Song,Yijian Xu,Cheng Li,Tingyan Ren,Bofeng Cai,Dahai Yang,Junhao Chen,Lewei Tong,Rui Huang,Edison Huixiang Ang,Xingqi Liao,Binghui Ge,Hongfa Xiang
标识
DOI:10.1016/j.est.2024.110578
摘要
The effective recycling of retired LiFePO4 batteries serves dual purposes: addressing the resource supply-demand contradiction and mitigating environmental pollution. However, the existing recycling methods for waste LiFePO4 batteries often entail high energy consumption, time consumption, complex procedures, or the use of substantial amounts of chemical raw materials, leading to increased recycling costs. Moreover, both methods generate toxic gases or discharge excessive pollutant-containing liquids during the recycling process, posing a risk of secondary pollution. Here, we introduce the application of ultrasound-assisted regeneration in waste LiFePO4 cathode material directly. Ultrasound waves generate localized high temperature, high pressure, and intense shock wave jets to repair the lithium vacancy defects and anti-site defects in the waste LiFePO4. Based on the experimental findings, the regeneration of LiFePO4 was achieved with impressive results. At an ultrasound power of 500 W and a duration of 50 min, the regenerated LiFePO4 displayed a discharge specific capacity of 135.1 mAh∙g−1 and an impressive capacity retention of 97 % after 100 cycles at a 1C (1C = 170 mA g−1) current density. This study presents a promising and environmentally friendly approach for recycling and regenerating retired LiFePO4 batteries.
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