分离器(采油)
材料科学
复合数
惰性
聚乙烯
涂层
化学工程
复合材料
锂离子电池
电化学
电极
化学
电池(电)
工程类
物理化学
物理
功率(物理)
有机化学
热力学
量子力学
作者
Shi Li,Yu Wu,Xiaoli Ma,Jiwen Hu,Qiusheng Song,Xianrong Shen,Wei Zhang
标识
DOI:10.1016/j.jpowsour.2023.233620
摘要
Lithium-ion batteries have received a great deal of attention on the world stage due to their high-power density and superior electronic properties. Herein, a novel phase change composite separator was successfully fabricated into lithium-ion battery cells by microfluidic technology. The phase change material composite separator was manufactured with polyethylene (PE) as the base film and employing the crystalline phase change property of polyethylene oxide (PEO). The phase change solution was atomized and delivered to the surface of the separator using high-pressure inert gases, and then crystallized on the separator substrate by controlling the temperature difference. The capacity retention and capacity recovery of the manufactured phase change material composite separator cells were 96.9% and 97.8%, respectively. In addition, the cells demonstrated superior multiplier performance (∼98% capacity retention at 1C). Additionally, the phase change material was introduced into the separator coating layer to increase the heat resistance of the separator, while the electrochemical performance was exceptional and the safety performance was favorable, thus alleviating the heat accumulation inside the battery at the source and effectively enhancing the safety of lithium-ion batteries.
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