Nanocellulose-graphene composites: Preparation and applications in flexible electronics

In recent years, the pursuit of high-performance nano-flexible electronic composites has led researchers to focus on nanocellulose-graphene composites. Nanocellulose has garnered widespread interest due to its exceptional properties and unique structure, such as renewability, biodegradability, and biocompatibility. However, nanocellulose materials are deficient in electrical conductivity, which limits their applications in flexible electronics. On the other hand, graphene boasts remarkable properties, including a high specific surface area, robust mechanical strength, and high electrical conductivity, making it a promising carbon-based nanomaterial. Consequently, research efforts have intensified in exploring the preparation of graphene-nanocellulose flexible electronic composites. Although there have been studies on the application of nanocellulose and graphene, there is still a lack of comprehensive information on the application of nanocellulose/graphene in flexible electronic composites. This review examines the recent developments in nanocellulose/graphene flexible electronic composites and their applications. In this review, the preparation of nanocellulose/graphene flexible electronic composites from three aspects: composite films, aerogels, and hydrogels are first introduced. Next, the recent applications of nanocellulose/graphene flexible electronic composites were summarized including sensors, supercapacitors, and electromagnetic shielding. Finally, the challenges and future directions in this emerging field was discussed.