等离子体子
谐振器
分裂环谐振器
光电子学
戒指(化学)
材料科学
近场和远场
光学
物理
纳米技术
化学
有机化学
作者
Yue You,Xiao-Jing Du,Lin Ma,Hua Qiu,Jun He,Zhong‐Jian Yang
出处
期刊:Nano Letters
[American Chemical Society]
日期:2025-06-06
被引量:1
标识
DOI:10.1021/acs.nanolett.5c02010
摘要
Plasmonic antennas generating strong near-field enhancement primarily rely on electric dipole resonance, a mechanism that also limits their further optimization. Here we propose an asymmetric split-ring resonator (ASRR) that induces differential charge distribution across the split gap. Through asymmetric structural modulation, charges are highly localized at the designated terminal, enabling efficient near-field enhancement. This configuration was initially developed via a hybrid framework integrating evolutionary optimization with residual neural networks and subsequently simplified into an ASRR prototype using Occam's Razor principle. The ASRR dimer demonstrates >6-fold electric-field intensity enhancement compared to conventional nanorod dimers at subwavelength scale, while exhibiting a superior Purcell factor and fluorescence enhancement. This breakthrough creates new opportunities in surface-enhanced spectroscopy and light-matter interactions.
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