Co-Benefits of Pollutant Removal, Water, and Heat Recovery from Flue Gas through Phase Transition Enhanced by Corona Discharge

烟气 电除尘器 烟气脱硫 热交换器 废物管理 电晕放电 化学 火力发电站 污染物 环境科学 环境工程 热力学 物理 工程类 物理化学 电极 有机化学
作者
Lingyu Shao,Yifan Wang,Can Zhou,Zhengda Yang,Wenchao Gao,Zhicheng Wu,Lianming Li,Yonglong Yang,Yang Yang,Chenghang Zheng,Xiang Gao
出处
期刊:Environmental Science & Technology [American Chemical Society]
卷期号:56 (12): 8844-8853 被引量:5
标识
DOI:10.1021/acs.est.2c00917
摘要

Pollutant removal and resource recovery from high-humidity flue gas after desulfurization in a thermal power plant are crucial for improving air quality and saving energy. This study developed a flue gas treatment method involving phase transition enhanced by corona discharge based on laboratory research and established a field-scale unit for demonstration. The results indicate that an adequate increase in size will improve the ease of particle capture. A wet electrostatic precipitator is applied before the condensing heat exchangers to enhance the particle growth and capture processes. This results in an increase of 58% in the particle median diameter in the heat exchanger and an emission concentration below 1 mg/m3. Other pollutants, such as SO3 and Hg, can also be removed with emission concentrations of 0.13 mg/m3 and 1.10 μg/m3, respectively. Under the condensation enhancement of the method, it is possible to recover up to 3.26 t/h of water from 200 000 m3/h saturated flue gas (323 K), and the quality of the recovered water meets the standards stipulated in China. Additionally, charge-induced condensation is shown to improve heat recovery, resulting in the recovery of more than 43.34 kJ/h·m3 of heat from the flue gas. This method is expected to save 2628 t of standard coal and reduce carbon dioxide emission by 2% annually, contributing to environmental protection and global-warming mitigation.

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