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Comprehensive Multidimensional Analysis of Metal(loid)-Containing Dust in Plastic Sports Facilities: Insights into the Potential Sources and Health Risks

环境化学 道路扬尘 健康风险 电感耦合等离子体质谱法 人类健康 环境科学 污染 化学 金属 冶金 质谱法 微粒 材料科学 环境卫生 有机化学 生态学 生物 医学 色谱法
作者
Xiangwei Tian,Qingqing Yang,Yuqian Zhao,Dandan Cao,Yanwei Liu,Yingying Guo,Wenbin Cui,Ligang Hu,Yongguang Yin,Yong Cai,Guibin Jiang
出处
期刊:Environmental Science & Technology [American Chemical Society]
卷期号:58 (52): 23212-23221 被引量:2
标识
DOI:10.1021/acs.est.4c11896
摘要

Dust released from widely established plastic sports courts and synthetic turf poses potential environmental and health risks. Herein, we systematically investigate the metal(loid) characteristics, potential sources, and health risks of 162 dust samples from 17 campuses in Beijing, using complementary analytical techniques. Bulk analysis revealed higher levels of Zn, Pb, Cu, Sb, Cd, and Cr than background values, suggesting excessive anthropogenic contamination. Pb and Cr in plastic basketball court and track dust and Zn and Sb in synthetic turf dust were higher than those in other sports facilities. Multielement single-particle inductively coupled plasma time-of-flight mass spectrometry (spICP-TOF-MS) revealed more Fe-, Al-, Si-, Ti-, and Pb-containing particles in the dust. At least 92% toxic Pb-containing particles were composed of multiple elements. The significant correlations between Pb and Cr contents on individual dust particles support their common potential source from inorganic pigments (crocoite, PbCrO4). Pb, Sb, As, and Cr in the dust pose higher health risks through intake. The risks were estimated to be approximately 3-5 times higher for children than for adults. Additionally, highly toxic Cr(VI) and As(III) species were observed in the sweat and gastric juice leachate of dust, highlighting severe threats of the metal(loid)s to human health.
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