材料科学
电极
复合材料
复合数
电镀(地质)
铜
表面粗糙度
电阻率和电导率
镀铜
电镀
图层(电子)
冶金
化学
电气工程
物理化学
地球物理学
地质学
工程类
作者
Jiahua Li,Aifen Tian,Xixi Wang,Aifen Tian,Xinrong Zhang,Bin Feng,Shanshan Yao,Huiling Du
出处
期刊:ACS omega
[American Chemical Society]
日期:2022-05-19
卷期号:7 (21): 17575-17582
被引量:4
标识
DOI:10.1021/acsomega.1c07319
摘要
As a kind of flexible intelligent driving material, ionic polymer-metal composite (IPMC) has attracted the attention of researchers due to its advantages of lightweight, large deformation, and fast response. However, the reciprocating bending of IPMC causes cracks to appear on the surface metal electrode layer and reduces the water uptake (WUP). At the same time, the metal particles are extruded, resulting in an increase in resistivity, which affects the driving performance of the materials. Therefore, in this study, considering the preparation cost, Cu-Pt-IPMC using Pt and Cu as a composite electrode with the self-healing system was prepared by electroless plating and Cu2+ was used as driving ions that can form a reversible circulation system with a copper electrode. The WUP, surface resistivity, and driving performance were tested and analyzed and the surface roughness was characterized by Matlab. The results show that the dendritic interface electrodes (DIEs) appear at the contact interface between the metal electrode and the film, which extend deeper and wider in the film with the increase in the cycles of autocatalytic platinum plating (ACP-Pt), and the output displacement and blocking force of 61.20 mm and 34.26 mN, respectively, have been achieved in the Cu-Pt-IPMC sample after three cycles of ACP-Pt. Based on these analyses, this study proves that the presence of Cu2+ can repair the cracked electrode on the surface of IPMC and reduce the surface electrode resistance, improving the driving performance.
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