光催化
半导体
能量转换
能量转换效率
催化作用
太阳能转换
纳米技术
材料科学
化学
过程(计算)
工艺工程
太阳能
生化工程
计算机科学
工程类
光电子学
物理
电气工程
有机化学
操作系统
热力学
作者
Zili Ma,Yihong Chen,Chao Gao,Yujie Xiong
出处
期刊:Energy & Fuels
[American Chemical Society]
日期:2022-06-24
卷期号:36 (19): 11428-11442
被引量:11
标识
DOI:10.1021/acs.energyfuels.2c01351
摘要
Converting earth-abundant CH4 to value-added feedstocks for chemical industry is an intriguing approach for utilization of carbon resource. However, the high inertness of CH4 makes its catalytic conversion one of the holy grails and suffers from intense energy consumption in a traditional conversion process. The recently developed semiconductor-based photocatalytic processes operated at mild conditions shine light on the way to achieve efficient CH4 conversion driven by only clean solar energy. In this review, we discuss the advancements in semiconductor-based photocatalytic CH4 conversion and highlight the roles of cocatalysts, which are the key components in hybrid photocatalysts, in augmenting catalytic performance. Furthermore, the future research efforts on cocatalysts are proposed for promoting photocatalytic CH4 conversion.
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