材料科学
纳米技术
碳纳米管
等离子体子
分子
纳米-
表面等离子共振
可穿戴计算机
光电子学
纳米颗粒
计算机科学
复合材料
化学
有机化学
嵌入式系统
作者
Dongzhen Chen,Jianzhao Gao,Dan He,Jingshun He,Li Yang,Meng Zhang,Wenya Li,Xin Chen,Xiaohui He,Tao Fu
标识
DOI:10.1021/acsami.2c22634
摘要
Wearable, noninvasive, and simultaneous sensing of subtle strains and eccrine molecules on human body is essential for future health monitoring and personalized medicine. However, there is a huge chasm between biomechanics and bio/chemical molecule detections. Here, a wearable plasmonic bridge sensor with multiple abilities to monitor subtle strains and molecules is developed. Hollow Au-Ag nano-rambutans and carbon nanotubes (CNTs) are adsorbed in the nonwoven fabrics (NWFs) conjointly, where the gap between the conducting network of CNTs is bridged by the Au-Ag nano-rambutans during the subtle strain sensing, and the detection sensitivity for stress is improved at least 1 order of magnitude compared to that with the only CNTs. In order to acquire the accurate human action recognition, a machine learning algorithm (support vector machines) based on output biomechanics data is designed. The average accuracy of our plasmonic bridge sensor reaches 89.0% for human action recognition. Moreover, due to the hollow structure and high nanoroughness, the single Au-Ag nano-rambutan particle has strong localized surface plasmon resonance effect and high surface-enhanced Raman scattering (SERS) activity. Based on their unique SERS spectra introduced by the hollow Au-Ag nano-rambutan adsorbed in the NWFs, noninvasive extraction and "fingerprint" recognition of bio/chemical molecules could be realized during the wearable sensing. In sum, the NWFs/CNTs/Au-Ag sensor bridges the barrier between the bodily strain detection and molecule recognition during the wearable sensing. Such integrated and multifunctional sensing strategy for universal biomechanics and bio/chemical molecules means to assess human health to be of importance.
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