Two birds with one stone: The multiple roles of hydrothermal treatment in dewatering municipal sludge and producing value-added products

Sludge dewatering and resource recovery are key steps in the sustainable treatment of municipal sludge (MS) owing to the high levels of moisture and nutrients. Among the treatment options available, hydrothermal treatment (HT) is promising to efficiently improve dewaterability and recover biofuels, nutrients, and materials from MS. However, hydrothermal conversion at different HT conditions generates multiple products. Integrating the characteristics of dewaterability and value-added products under different HT conditions facilitates the application of HT for the sustainable management of MS. Therefore, a comprehensive review of HT for its multiple roles in MS dewatering and value-added resource recovery is conducted. First, the impact of HT temperature on sludge dewaterability and key mechanisms are summarized. Then, this study elucidates the characteristics of biofuels produced (combustible gases, hydrochars, biocrudes, and H2-rich gases), nutrient recovery (proteins and phosphorus), and value-added materials under a wide range of HT conditions. Importantly, along with the integration and evaluation of HT product characteristics under different HT temperatures, this work proposes a conceptual sludge treatment system that integrates the different value-added products in different HT stages. Furthermore, a critical evaluation of the knowledge gaps in the HT for sludge deep dewatering, biofuels, nutrients, and materials recovery is provided along with recommendations for further research.