化学工程
电催化剂
碳纤维
塔菲尔方程
过电位
电化学
作者
Saerom Ohn,Seung Yeon Kim,Seon Kyu Mun,Junghoon Oh,Young Jin Sa,Sunghee Park,Sang Hoon Joo,Seong Jung Kwon,Sungjin Park
出处
期刊:Carbon
[Elsevier]
日期:2017-11-01
卷期号:124: 180-187
被引量:43
标识
DOI:10.1016/j.carbon.2017.08.039
摘要
Hybrid materials containing single atoms or molecule-based active species immobilized on nanomaterials have been suggested as new, efficient catalytic systems for various reactions. In this study, novel hybrid materials consisting of molecularly dispersed Ni-based species on a graphitic carbon nitride (g-C3N4) framework are prepared, and their excellent electrocatalytic performance for the oxygen evolution reaction (OER) is discussed. Extensive chemical and structural characterizations confirm that the Ni-based species are attached and well-dispersed on the C3N4 network without agglomeration. In addition, results obtained from electrochemical characterization suggest that Ni-containing molecular entities dispersed on the C3N4 network are active species for the OER.
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