Achieve high-efficiency long afterglow luminescence control using CsPbI3 quantum dots

The construction of visible full-spectrum tunable afterglow luminescence is of great significance for long afterglow materials. Here we developed a new composite material whose afterglow were continuously tunable from blue to red light, we prepared CsPbI3 quantum dots (QDs) by thermal injection method and added passivators to obtain relatively more stable QDs materials, the SDS-CsPbI3 QDs after passivation treatment was more than twice the photoluminescent (PL) intensity of the original QDs after 10 days, which has a positive effect on the large-scale production and application of all-inorganic perovskite QDs. By uniformly distributing CsPbI3 QDs on the surface of Sr2MgSi2O7:Eu2+,Dy3+(SMS) by Stöber method, a color-tunable long-persistence luminescent material CsPbI3/[email protected]2 was prepared, and the tunable afterglow glows from 465 nm to 700 nm was realized by optical conversion. In addition, the PL intensity of the composite material under ultraviolet light is increased by more than 50%, and it can remain stable for a long time; its high temperature resistance is also improved to 140 °C; and the luminous intensity after 10 days remains at a high level. This research also provides new ideas and methods for the development of multicolor long afterglow materials.