激光阈值
材料科学
纳米线
卤化物
光电子学
钙钛矿(结构)
激光器
半导体激光器理论
增益开关
半导体
锡
宽禁带半导体
激发
光子学
光抽运
纳米激光器
纳米光子学
自发辐射
激光泵浦
作者
Yueran Zhao,Jingyi Zhu,Lin Chen,Zhuo Xue,Fuying Wang,Xiaotian Fang,Haobo Zhang,Zhengyuan Zhang,Qiuchen Zhao,Enge Wang,Minliang Lai
出处
期刊:Nano Letters
[American Chemical Society]
日期:2026-09-23
卷期号:26 (41): 14341-14350
标识
DOI:10.1021/acs.nanolett.6c03883
摘要
Abstract Tin halide perovskites are promising lead-free optical gain media, yet stable quasi-continuous-wave/continuous-wave (quasi-CW/CW) lasing remains challenging under practical operating conditions. Here, we demonstrate robust quasi-CW lasing from single-crystalline CsSnBr3 nanowires under ambient conditions. Under quasi-CW excitation, these nanowires exhibit a low threshold of 64.5 μJ cm–2, markedly lower than that of representative III–V and II–VI semiconductor nanowires. Moreover, the CsSnBr3 nanowire lasers sustain lasing under repeated quasi-CW excitation in air for over 60 min. We further achieve wide wavelength-tunable lasing from 704 to 974 nm by Br/I alloying. In addition, we observe exciton–polariton (EP) formation and pronounced excitation-dependent blueshifts of the lasing emission, suggesting a polaritonic contribution to the low-threshold quasi-CW lasing process. These results establish tin halide perovskite nanowires as a robust, wavelength-tunable platform for quasi-CW nanolasers and support their potential for future CW nanolasers and integrated photonics.
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