Comparing CO2 and Variable-TDS Waste-Fluid Injection Into Deep Saline Geologic Formations

盖层 地质学 超压 诱发地震 羽流 石油工程 地球化学 卤水 碳酸盐 固碳 注入井 岩石学 二氧化碳 材料科学 化学 物理 地震学 冶金 热力学 有机化学
作者
Esmail Ansari,Yevhen Holubnyak,Franciszek Hasiuk,Jennifer Raney
出处
期刊:Frontiers in Energy Research [Frontiers Media]
卷期号:10 被引量:1
标识
DOI:10.3389/fenrg.2022.864013
摘要

There is a renewed interest in carbon capture, utilization, and storage technology due to recently expanded US Internal Revenue Service 45Q credits as well as to reduce anthropogenic carbon emissions to the atmosphere. Deep carbonate reservoirs in western Kansas have the potential for CO 2 storage because they have experienced low waste-fluid injection volumes to date. Waste-fluid injection in Kansas has not caused felt seismicity for more than seven decades. However, beginning in 2013, the state has experienced increased seismicity due to increased subsurface pressure associated with the injection of large volumes of variable-TDS (total dissolved solids) waste-fluid in US EPA Class I and Class II wells. This work compares CO 2 , low-TDS, and high-TDS injection practices and quantifies the induced spatial and temporal patterns in overpressure in the caprock, reservoir, and its hydraulically connected crystalline basement, where the majority of induced seismicity in Kansas has been observed. Our results show that pressure buildup is higher in the caprock and lower in the crystalline basement when injecting CO 2 as compared to variable-TDS waste-fluid injection. The CO 2 plume tends to expand at the top of the reservoir, primarily due to its lower density and viscosity than reservoir brines, creating an overpressure plume that moves the resident brine across the caprock. In contrast, waste-fluid injection moves more resident brine down into the basement, particularly when high-TDS waste-fluid is injected. This result is particularly valid for high-permeability carbonate reservoirs, in which gravity forces dominate over viscous forces and move the CO 2 and overpressure plume toward the top of the reservoir. Our study may explain the lack of human-perceivable induced seismicity at operating CO 2 injection projects globally.

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