Strong coupling of excitons in a two-dimensional atomic crystal with quasi-bound state in the continuum supported by a single nanoparticle

激子 纳米颗粒 材料科学 束缚态 比克西顿 联轴节(管道) 凝聚态物理 分子物理学 单晶 原子物理学 化学物理 物理 纳米技术 化学 结晶学 量子力学 冶金
作者
Qi Ding,Xun Zhou,Peng Xie,Shiyu Shen,Ling Yue,Hong Zhang,Wei Wang
出处
期刊:Applied Physics Letters [American Institute of Physics]
卷期号:126 (8)
标识
DOI:10.1063/5.0250193
摘要

Bound states in the continuum (BICs) supported by high-index dielectric nanoparticles have garnered significant attention due to their ability to achieve subwavelength confinement with high-quality factors, offering great potential for both fundamental studies of light–matter interactions and the development of compact photonic devices. However, the strong coupling of BICs with quantum emitters in single-particle systems has not been reported. In this paper, we propose a dielectric nanodisk integrated with a monolayer of transition metal dichalcogenides. A supercavity mode known as Friedrich–Wintgen BIC is launched in the nanodisk to enable strong coupling of BIC with WS2 excitons. We demonstrate that the reduction in coupling strength as the quasi-BIC quality factor increases is due to a decrease in the number of excitons participating in the coupling. Additionally, the coupling strength can be manipulated by adjusting the shape and aspect ratio of the nanoresonators, enabling a transition from strong to weak coupling regimes. Near-field analysis shows that the manipulation of the BIC–exciton interaction arises from the overlap of the BIC mode's near-field with the excitons. Our findings offer a promising strategy for manipulating light–matter interactions and enhance the potential applications of BIC resonances in photonics.
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