Synergistic barium titanate/MXene composite as a high-performance piezo-photocatalyst for efficient dye degradation

降级(电信) 罗丹明B 钛酸钡 光催化 复合数 材料科学 纳米颗粒 化学工程 紫外线 纳米技术 陶瓷 复合材料 化学 催化作用 光电子学 计算机科学 有机化学 电信 工程类
作者
Linghui Meng,Lu Zhou,Chao Liu,Haowei Jia,Yile Lu,Dali Ji,Tianyue Liang,Yuan Yu,Xinren Zhang,Yanzhe Zhu,Yue Jiang,Peiyuan Guan,Yingze Zhou,Qi Zhang,Tao Wan,Mengyao Li,Zhi Li,Rakesh Joshi,Zhaojun Han,Dewei Chu
出处
期刊:Journal of Colloid and Interface Science [Elsevier BV]
卷期号:674: 972-981 被引量:32
标识
DOI:10.1016/j.jcis.2024.06.222
摘要

Piezo-photocatalysis combines photocatalysis and piezoelectric effects to enhance catalytic efficiency by creating an internal electric field in the photocatalyst, improving carrier separation and overall performance. This study presents a high-performance piezo-photocatalyst for efficient dye degradation using a synergistic barium titanate (BTO)-MXene composite. The composite was synthesized via a facile method, combining the unique properties of BTO nanoparticles with the high conductivity of MXene. The structural and morphological analysis confirmed the successful formation of the composite, with well-dispersed BTO nanoparticles on the MXene surface. The piezo-photocatalytic activity of the composite was evaluated using a typical dye solution (Rhodamine B: RhB) under ultraviolet irradiation and mechanical agitation. The results revealed a remarkable enhancement in dye degradation (90 % in 15 min for piezo-photocatalysis) compared to individual stimuli (58.2 % for photocatalysis and 95.8 % in 90 min for piezocatalysis), highlighting the synergistic effects between BTO and MXene. The enhanced catalytic performance was attributed to the efficient charge separation and transfer facilitated by the composite's structure, leading to increased reactive species generation and dye molecule degradation. Furthermore, the composite exhibited excellent stability and reusability, showcasing its potential for practical applications in wastewater treatment. Overall, this work represents a promising strategy for designing high-performance synergistic catalysts, addressing the pressing need for sustainable solutions in environmental remediation.
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