材料科学
电池(电)
功率密度
分解水
化学工程
碳纤维
碳纳米管
纳米技术
析氧
超级电容器
多孔性
电极
电流密度
催化作用
复合材料
功率(物理)
电化学
复合数
化学
物理化学
物理
量子力学
光催化
工程类
生物化学
作者
Lei Yan,Zhuying Xu,Xunan Liu,Sajid Mahmood,Junling Shen,Jiqiang Ning,Sha Li,Yijun Zhong,Yong Hu
标识
DOI:10.1016/j.cej.2022.137049
摘要
A structural engineering strategy is proposed to fabricate trifunctional electrocatalysts supported by carbon cloth, composed of NiFe-LDH nanosheets aligned on Co-embedded N-doped carbon triangle plates with interwoven carbon nanotubes (Co@NC-CNTs@NiFe-LDH), which is employed as a freestanding electrode for both flexible Zn-air batteries and self-powered water splitting. This unique 3D hierarchical structure and the strong interfacial coupling between the NiFe-LDH and Co@NC-CNTs facilitate the transport of oxygen species as well as electrons and achieve synergy between the integrated nano-scaled structures with different functional components. As expected, a large peak power density of 194 mW cm−2 and outstanding durability for 760 h are obtained in the as-assembled rechargeable Zn-air battery. The resultant water splitting device acquires a cell voltage of 1.66 V at 10 mA cm−2 and the as-assembled Zn-air battery has been successfully employed in a self-power water splitting system, demonstrating a great potential prospect for practical renewable energy applications.
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