甲醛
氮化硼
催化作用
材料科学
化学工程
催化氧化
气凝胶
多孔性
无机化学
吸附
化学
纳米技术
有机化学
复合材料
工程类
作者
Dongyun Chen,Guping Zhang,Mengmeng Wang,Najun Li,Qingfeng Xu,Hua Li,Jinghui He,Jianmei Lu
标识
DOI:10.1002/anie.202013667
摘要
Abstract The catalytic room temperature oxidation of formaldehyde (HCHO) is widely considered as a viable method for the abatement of indoor toxic HCHO pollution. Herein, Pt/MnO 2 nanoflowers anchored to boron nitride aerogels (Pt/MnO 2 ‐BN) were fabricated for the catalytic room temperature oxidation of HCHO. The three‐dimensional Pt/MnO 2 ‐BN aerogels demonstrated superior catalytic activity as a result of the improved diffusion of the reactant molecules within the porous structure. Furthermore, the porous aerogels displayed excellent HCHO adsorption capacities, which promote a rapid HCHO gas‐phase concentration reduction and a subsequent complete oxidation of the adsorbed HCHO. The combined adsorption and oxidation properties of the Pt/MnO 2 ‐BN aerogels enhance the oxidative removal of HCHO. The optimized Pt/MnO 2 ‐BN demonstrated excellent catalytic activity toward HCHO (200 ppm) at room temperature, achieving a 96 % formaldehyde conversion after 50 min.
科研通智能强力驱动
Strongly Powered by AbleSci AI