光催化
制氢
材料科学
三元运算
催化作用
氢
异质结
可见光谱
化学工程
纳米技术
光电子学
化学
计算机科学
有机化学
工程类
程序设计语言
作者
Yingrui Wang,Chao Liu,Cui Kong,Fengjun Zhang
标识
DOI:10.1016/j.colsurfa.2022.129746
摘要
The addition of a co-catalyst is one of the most effective ways to enhance the performance of CdS photocatalytic hydrogen production. In this work, ternary photocatalysts with Defect MoS2 and Ti3C2 acting synergistically on CdS are explored. The experimental results showed that the Defect MoS2/Ti3C2/CdS photocatalyst had excellent photocatalytic hydrogen production performance of 14.1 mmol h−1g−1, which was 18.5, 12.4, and 1.2 times higher than that of CdS, Ti3C2/CdS and Defect MoS2/CdS, respectively. Defect MoS2 and Ti3C2 synergistically interact with CdS and form heterojunctions, which improve the carrier separation efficiency and effectively suppress the recombination of photogenerated carriers. A possible photocatalytic hydrogen production mechanism of Defect MoS2/Ti3C2/CdS is also proposed. The dual co-catalysts of Defect MoS2 and Ti3C2 demonstrated in this paper provide a feasible approach for the development of composite catalysts.
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