量子点
X射线光电子能谱
光催化
材料科学
异质结
光电子学
光降解
甲基橙
光致发光
光谱学
透射电子显微镜
吸收(声学)
分析化学(期刊)
光化学
纳米技术
化学
化学工程
催化作用
物理
复合材料
有机化学
工程类
量子力学
作者
Hui Wang,Xingzhong Yuan,Hou Wang,Xiaohong Chen,Zhibin Wu,Longbo Jiang,Weiping Xiong,Guangming Zeng
标识
DOI:10.1016/j.apcatb.2016.03.075
摘要
In recent years, exploiting novel photocatalysts with a broad range of wavelengths photoresponse is undoubtedly interesting in photocatalytic field. Here, a novel Sb2S3/ultrathin g-C3N4 sheets heterostructures embedded with g-C3N4 quantum dots (CNS) was successfully fabricated via a facile hydrothermal process. The samples were systematically characterized by the field emission scanning electron microscopy (FESEM), transmission electron microscopy (TEM), X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), UV–vis-NIR diffuse reflection spectroscopy (UV-vis-NIR DRS) and photoluminescence (PL) spectroscopy. It is indicated that the composites have fast electron transport and enhanced solar light absorption. Moreover, the CNS composite exhibits a significant photoelectric conversion property in near-infrared (NIR) wavelength range. The photocatalytic activities of the samples were evaluated by the degradation of methyl orange (MO) upon NIR irradiation. The photodegradation rate of the optimal CNS for MO was 0.0103 min−1, about 2.6 times higher than that of pure Sb2S3. The improved NIR photocatalytic activity may base on the improved absorption in the NIR region, efficient electron-hole separation and the up-converted PL property of g-C3N4 quantum dots (CNQD).
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