富勒烯
光催化
分解水
光催化分解水
试剂
材料科学
图层(电子)
带隙
纳米技术
化学工程
化学
光电子学
物理化学
催化作用
有机化学
工程类
作者
Taotao Wang,Li Zhang,Jinbao Wu,Muqing Chen,Shangfeng Yang,Yalin Lu,Pingwu Du
标识
DOI:10.1002/anie.202311352
摘要
Abstract A few‐layer fullerene network possesses several advantageous characteristics, including a large surface area, abundant active sites, high charge mobility, and an appropriate band gap and band edge for solar water splitting. Herein, we report for the first time that the few‐layer fullerene network shows interesting photocatalytic performance in pure water splitting into H 2 and H 2 O 2 in the absence of any sacrificial reagents. Under optimal conditions, the H 2 and H 2 O 2 evolution rates can reach 91 and 116 μmol g −1 h −1 , respectively, with good stability. This work demonstrates the novel application of the few‐layer fullerene network in the field of energy conversion.
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