正渗透
膜
渗透
聚酰胺
聚砜
海水淡化
化学工程
化学
图层(电子)
膜技术
材料科学
色谱法
反渗透
渗透
纳米技术
高分子化学
生物化学
工程类
作者
Nur Diyana Suzaimi,Pei Sean Goh,Kar Chun Wong,Takaaki Taniguchi,Jun Wei Lim,Nik Ahmad Nizam Nik Malek,Ahmad Fauzi Ismail
标识
DOI:10.1016/j.seppur.2023.125401
摘要
To realize nutrient (NO3–-N and PO43−-P) enrichment through FO, this study focuses on tailoring polysulfone (PSF) support layer of TFC FO membrane using 1D akaganeite (Ak) as nano-template to improve the permeance and selective separation of nutrient ions. The incorporation and the subsequent removal of the nano-template from the PSF support layer instantly created porous structures with the desired nanochannel architectures. The separation performance of the resultant e-Ak/TFC membrane is superior to other as-synthesized TFC membranes due to the presence of highly permeable channels, lower membrane tortuosity of support layer and the formation of homogenous polyamide active layer. This restricts the back-diffusion of ions in the support layer, hence improving the effective driving force across the layer. The membrane demonstrated increased water flux from 6.5 for control TFC to 14.1 L/m2∙h for e-Ak/TFC membrane (∼2.2 times higher) along with high selectivity, JW/JS of 0.58 g/L and lower S value. NO3–-N and PO43−-P were effectively enriched in the feed side due to high ion removal efficiencies by the membrane (>97 %) with water reduction of approximately 25 %. We anticipate this work offers an insight into the design of FO membrane that is capable for desalination and enrichment of nutrient in wastewater.
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