Selective detection of trace carbon monoxide at room temperature based on CuO nanosheets exposed to (111) crystal facets

一氧化碳 检出限 材料科学 氧气 选择性 热液循环 Crystal(编程语言) 碳纤维 纳米技术 化学工程 化学 复合材料 色谱法 有机化学 计算机科学 复合数 工程类 程序设计语言 催化作用
作者
Yuanyuan Wu,Ji Li,Ming-Song Lv,Xian‐Fa Zhang,Rui Gao,Chuanyu Guo,Xiaoli Cheng,Xin Zhou,Yingming Xu,Shan Gao,Zoltán Major,Li-Hua Huo
出处
期刊:Journal of Hazardous Materials [Elsevier BV]
卷期号:442: 130041-130041 被引量:79
标识
DOI:10.1016/j.jhazmat.2022.130041
摘要

In recent years, carbon monoxide (CO) intoxication incidents occur frequently, and the sensitive detection of CO is particularly significant. At present, most reported carbon monoxide (CO) sensors meet the disadvantage of high working temperature. It is always a challenge to realize the sensitive detection of carbon monoxide at room temperature. In this study, CuO nanosheets exposed more (111) active crystal facets and oxygen vacancy defects were synthesized by a simple and environmentally friendly one-step hydrothermal method. The sensor has good comprehensive gas sensing performance, compared with other sensors that can detect CO at room temperature. The response value to 100 ppm CO at room temperature is as high as 39.6. In addition, it also has excellent selectivity, low detection limit (100 ppb), good reproducibility, moisture resistance and long-term stability (60 days). This excellent gas sensing performance is attributed to the special structural characteristics of 2D materials and the synergistic effect of more active crystal facets exposed on the crystal surface and oxygen vacancy defects. Therefore, it is expected to become a promising sensitive material for rapid and accurate detection of trace CO gas under low energy consumption, reduce the risk of poisoning, and then effectively protect human life safety.
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