荧光
光致发光
材料科学
碳纤维
热解
量子点
发光
纳米技术
机制(生物学)
带隙
共轭体系
光化学
光电子学
化学
聚合物
光学
有机化学
物理
复合材料
复合数
量子力学
作者
Yan Li,Can Liu,Hao Sun,Menglin Chen,Defa Hou,Yunwu Zheng,Haijiao Xie,Bei Zhou,Xu Lin
标识
DOI:10.1002/advs.202300543
摘要
Abstract Reported in 2004, carbon dots (CDs) have been widely used in various fields due to their excellent optical properties. However, the mechanism of their fluorescence modulation is still a controversial issue, which also seriously affects the further development of carbon dots. In this paper, m ‐hydroxybenzaldehyde is used as a raw material to obtain multicolor luminescent CDs by pyrolysis under different reaction conditions, thereby revealing the forbidden band tuning and formation mechanism of CDs. Different acid–base conditions lead to different reaction paths of the precursors, forming molecular fluorophores with different conjugated structures, which aggregate to eventually form CDs and further enhance the photoluminescence of the system by inhibiting the movement of the fluorescent centers.
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